If you do a search you will find other threads on this same topic.
I've done more than a few freedives in a drysuit. DUI TLS-350 with C4 thinsulate worked the best- easy to move around in and let me get deeper than with other suits. I was able to get down about 30'-35' before the squeeze got so bad I couldn't move around that well. If I were just riding a scooter I might have been able to go deeper- since I wouldn't have to kick at all.
I've also used 7mm neoprene drysuits- which have huge buoyancy shifts and I never cared for them much. I've also done it with my old CF200 (crushed neoprene) drysuit- which yielded better results than the 7mm suit, but no where near as nice as with the tri-lam.
The worst luck I had was with a Viking suit while wearing the Viking foam underwear- only able to get down 25' before the squeeze got to me. It's an awesome suit for scuba diving in crappy water, but not the best freediving suit.
It's possible freedive in a drysuit, but a real freediving wetsuit will work much better- and scuba wetsuits pretty much suck for warmth, or anything else. A real freediving wetsuit will also work out well for scuba dives to a certain extent. For the water I dive in I have no problem using a freediving wetsuit for any no-deco scuba dive. If I'm going into deco, which is pretty much any time bother to strap a tank(s) onto my back I wouldn't want to go below 70' with one. This would change in warmer water, but I'm talking 40F local stuff.
For drysuit diving I really like Esclapez/Immersion openheel freediving fins- in black. They also make a green version and have a couple of choices in footpocket sizes. I have no issues getting a size 10 drysuit boot, with socks and booties, into a pair of XL fins with room to spare.
Oh, and I'd skip the bottle to add on for suit inflation to get a bit deeper- you'll end up blowing the gas in no time with all the up and down stuff that you'll be doing. I will say that another instructor I used to teach with liked to freediving down to a platform at 25' in his neoprene drysuit and wrap his knees around the rail while he filled his suit with a tank lying on the bottom. After disconnecting the suit he would let her rip and launch himself out of the water- people get pretty bored diving in the same quarries all the time.rofl
Jon